It’s as simple as that.
Make the other 2 bosses drop Duriel mats.
That would not only make them more desirable to do but alleviate the bottle neck of Varshan and Grigoire being all that matters.
Yeah, it is rather strange that two bosses provide access to the Uber, while two are essentially useless after getting whatever uniques you’d like off their corpses. Still, the actual amount of Living Steel you get during the Helltides is too low for time spent compared with what it takes to accumulates Varshan mats. The imbalance is too obvious to remain that way. 
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What needs to happen is -
Example: Post World Boss kill 1-3 Monsters are ‘called forth’ and manifest.
Each can drop 1 - x Materials.
These “summons” can also appear at Legions, Helltides and randomly(had them many times in Vamptides).
Allow for Living Steel to have a chance to drop from them.
Other than sweeping Helltide changes, this will supplement to a degree without being as common as the other components(mid ground between their design philosophyand players wanting to be swimming in Living Steel)
Please tell me your name is a throw back to TMNT.
I agree with you, would give us a reason to continually farm the other bosses after we’ve essentially gotten the uniques we’ve wanted from them. I don’t count Uber Uniques just like I never counted them before we could “target farm” them. Their idea of target farming an Uber Unique is my idea of finding a winning lottery ticket where 1 billion play instead of 5 billion.
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And I imagine it should be so hard to do. I’m no programmer, but it sounds like a quick loot table adjustment.
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