My favorites are the ones that I use.
Of the Black Harvest
&
The Faceless One
The one that I don’t have but I love quite a bit is The Insane. Someday I’ll sit down and figure out how to get that… 
Slayer of Stupid, Incompetent and Disappointing Minions
But since I can’t use that outside of Blackwing Descent, I usually go with Brewmaster since that’s one of my IRL hobbies.
Lord of War. Close 2nd, Bloodthirsty
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-Undying
-Field Medic
-Knight-Captain
The loathsome DUNG-EATER!
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“Jenkins” by far.
I got it early on and it actually wasn’t easy. It was so much fun to see the video and then run into the room the same way.
Second place, “The crazy cat lady”
Hand of A’dal
Sounds sinister even tho it’s not
of The Black Harvest
Vanquisher. It’s so rare I have never seen anyone else with it.
Favorite one I use is Salty.
My favorite is any rank 1 PvP title. Ones I will never have hah.
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The one I want (Sapper) isn’t available, so I bounce between Highlord, the Explorer, and Ambassador.
ETA: I also like “the Argent Crusader.” Might even be the one I’m proudest of, since it required grinding to Exalted with both the Argent Dawn and the Argent Crusade.
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Depends on the toon, for me. My paladin, I like using Crusader, my warlock in his absolutely great transmog, it’s The Fabulous.
My warlock is Baroness ______, from Necrolord rep. Seems to fit her. The rest of my toons no title.
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I have the “of the black harvest” title, back then I specifically leveled up a warlock to get it, but I never use it because for every warlock I’ve ever had I just, for some reason, lose interest in the character and either delete them after getting them to max level or somewhere along the way.
Seeker of Knowledge, that I have yet to earn.
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That reminds me! I love the “Seeker ____” title
(was it “____ the Seeker” ??)
I use the of lordaeron one you don’t see it to much
Soupervisor makes me giggle.
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Crazy Cat Lady (because… well…yeah)
The Patient (because I’m not)
Salty (cuz I’m a sailor)
One of my toons is named Até, the Crazy Cat Lady
What funny about Até, she’s a Worgen.
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Conquerer or Azeroth
I had to start so many pvp wars to get it, those quest givers had it coming